- Myddelton family of Chirk Castle: estate papers and map collection (Chirk Castle Archive)
- William Henry Davies, Poet and Author: corresp with Lawrence Hockey and C. F. Cazenove 1908-1938 (NLW MS 23937)
- Roger Nicholas Edwards, Baron Crickhowell of Pont Esgob, politician: parliamentary papers incl corresp, speeches and printed items c1960-1999 (Lord Crickhowell Papers)
- Edmund Boleslaw Fryde, Professor of History: corresp and papers (E.B. Fryde Papers)
- John Gwyn Griffiths, Poet, Critic and Scholar: corresp and papers (Papurau J. Gwyn Griffiths)
- Michael Holroyd, biographer: original draft manuscript of the biography of Augustus John (Michael Holroyd Research Papers)
- Jeremy Hooker, Poet and Critic: corresp and typescripts (Jeremy Hooker Papers)
- John N Hutchinson, Emeritus Professor of Engineering: papers and corresp rel to the Aberfan disaster 1966-1967 (Professor J. N. Hutchinson: Aberfan Inquiry Papers)
- Jonah Jones, sculptor: letters (mainly to Dr Raymond Garlick) 1955-2003 (NLW MS 23936)
- Ceri Giraldus Richards, Painter: papers, artworks, photographs and printed items (Ceri Richards Papers)
- George Emlyn Williams, Playwright and Actor: papers incl corresp and photographs (NLW ex 2395)
- William Llewelyn Williams, Liberal MP, Barrister and Author: papers incl corresp and diaries (William Llewelyn Williams Papers)
- CND (Campaign for Nuclear Disarmament): Cymru: additional minutes, corresp and papers c1990-2004 (CND Cymru Papers)
- Edward Lhuyd, Celtic scholar and naturalist: letter to Humphrey Humphreys, bishop of Bangor, discussing fossils and Welsh manuscripts 1698 (NLW MS 23925)
- William Mathias, composer: two music manuscripts, 'In Arcadia' and 'Symphony No. 3' (William Mathias Archive)
- a catalogue of the representatives in Parliament for the counties and boroughs in Wales 1542-1747 (NLW MS 23938)
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National Library of Wales: Department of Collection Services