- Rhys Davies (1903-78), writer (addnl): papers (NLW MSS 23847-8)
- Menna Patricia Gallie (1920-90), author: corresp and papers (Menna Gallie Papers (Archif Menywod Cymru))
- Peter Hellings (1921-94), poet: papers (Peter Hellings Papers)
- Josef Charles Holbrooke (1878-1958), musician: ms of his opera 'Bronwen' (NLW MSS 23863-5E)
- Michael de Courcy Fraser Holroyd (b 1935), writer: corresp and research papers rel to Augustus John (Michael Holroyd (Augustus John) Papers)
- Augustus Edwin John (1878-1961), painter and etcher (addnl): appointment diaries and corresp (NLW MSS 23850-2, 23853-6)
- Gwen John (1876-1939), painter (addnl): corresp (NLW MSS 23850-2)
- Thomas Jones (1743-1803), landscape painter: memoirs and accounts (NLW MSS 23811E-12D)
- David Lloyd (1912-69), singer: papers (David Lloyd Papers)
- John Cowper Powys (1872-1963), author: letters to Margaret Moon (NLW MS 23862D)
- Nassau William Senior (1790-1864), economist: letters to him (NLW MSS 23857-61)
- Dewi-Prys Thomas (1916-85), head of the Welsh School of Architecture, Cardiff: corresp and plans rel to the design of the Gwynedd County Offices in Caernarfon (Dewi-Prys Thomas Papers)
- John Powell Ward (b 1937), poet and critic: papers rel to his period as editor of Poetry Wales (John Powell Ward (Poetry Wales) Papers)
- Welsh Amateur Music Federation: records 1970-2000 (Welsh Amateur Music Federation Records)
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National Library of Wales