- Donald Richard Coleman, Labour MP: political papers 1964-91 (Donald Coleman Papers)
- William Martin Condry (1918-1998), naturalist and writers: papers (William Condry Papers)
- Ellis William Davies (1871-1939), Liberal MP (addnl): corresp and papers (Ellis W Davies Papers)
- William Henry Davies, poet: corresp and papers 1905-38 (NLW MSS 23762-3D)
- John Elwyn (1916-1997), painter: corresp and papers (NLW MSS 23797-804)
- Raymond Garlick, author, critic and Welsh nationalist: diaries and notebooks 1987-98 (NLW MSS 23766-79)
- Sir William Goscombe John (1860-1952), sculptor: papers (NLW MSS 23749-50)
- Sir Charles Groves (1915-1992), conductor: papers (Sir Charles Groves Papers)
- Ray Howard-Jones (1903-1996), artist: papers (Ray Howard-Jones Papers)
- Berta Ruck (1878-1978), novelist (addnl): papers incl notebooks (MSS 23699, 23715-27, 23733-46, 23780-3, Berta Ruck)
- Caitlin Thomas, wife of Dylan Thomas: letters 1945-54 (NLW MS 23764E)
- Vernon Phillips Watkins (1906-1967), poet: papers incl drafts of poems (NLW MSS 23752-61)
- Henry Clarence Whaite (1828-1912), painter: papers (Clarence Whaite Papers)
- Rhydwen Williams (1916-1997),poet, novelist and minister: papers (Papurau Rhydwen Williams)
- Association of Visual Arts in Wales (formerly the Association of Artists and Designers in Wales): records incl accounts c1974-98 (Association of Artists and Designers in Wales)
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National Library of Wales