- William Ambrose Bebb (1894-1955), writer and historian: papers (Papurau W Ambrose Bebb)
- Cliff Bere, Welsh nationalist: papers c1940-95 (Cliff Bere Papers)
- Cardiff Bay Opera House Trust: records incl minutes 1991-97 (Cardiff Bay Opera House Trust Archive)
- Cardiff Roman Catholic Archdiocese: records 1850-1916 (Catholic Records: Dioceses of Newport and Menevia)
- Conservative Party (Wales): records 1937-97 (Conservative Party (Wales) Records)
- Football Association of Wales: minutes 1893-1986 (Football Association of Wales Records)
- Cledwyn Hughes, Baron Cledwyn of Penrhos, politician (addnl): papers 1944-97 (Lord Cledwyn of Penrhos Papers)
- Augustus Edwin John (1878-1961), painter and etcher (addnl): corresp (NLW MS 23697B)
- Glyn Jones (1905-95), poet, short story writer and novelist (addnl): literary manuscripts, corresp and papers (Glyn Jones Papers)
- Robert Maynard Jones (b1929), writer, critic and scholar: corresp and papers (Papurau Bobi Jones)
- Richard Dafydd Vivian Llewellyn Lloyd, novelist as Richard Llewellyn: letters 1944-45 (NLW MS 23710D)
- South Wales Football Association: minutes 1892-1962 (South Wales and Monmouthshire Football Association)
- Gwyn Thomas (1913-81), novelist, short story writer and playwright (addnl): papers (Gwyn Thomas MSS & Papers)
- Philip Edward Thomas, poet and prose writer: letters to Jesse Berridge 1901-17 (NLW MS 23695E)
- Thomas George Thomas, Viscount Tonypandy (1909-97), speaker of the House of Commons (addnl): papers (Viscount Tonypandy Papers)
- Welsh Town Planning and Housing Trust: records 1897-1977 (Welsh Town- Planning and Housing Trust Records)
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