- Meg Elis, writer: diaries 1968-2004 (Papurau Meg Elis)
- Alun Hoddinott (b 1929) composer: music MSS (Alun Hoddinott Archive)
- D Tecwyn Lloyd, writer and literary critic: papers 20th Cent (Papurau D Tecwyn Lloyd)
- John Cowper Powys, novelist and writer: papers (John Cowper Powys Papers)
- James Price, civil engineer: MSS, plans, photographs and printed papers (James Price Collection)
- Morgan Goronwy Rees, writer and university principal: additional papers (Goronwy Rees Papers)
- Graham Vivian Sutherland, painter: additional papers (Graham Sutherland Papers)
- Mary Taubman, writer: research papers on the artist Gwen John (Mary Taubman Papers)
- Urien Wiliam, writer and dramatist: papers (Papurau Dr Urien Wiliam)
- Qualifications, Curriculum and Assessment Authority for Wales: papers 1997-2006 (ACCAC Papers)
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National Library of Wales: Department of Collection Services