- Gillian Clarke (b 1937), poet: literary papers (Gillian Clarke Papers)
- Kenneth Harding (1903-92), composer and viola player: music manuscripts (Kenneth Harding Music Manuscripts)
- David Martyn Lloyd-Jones (1899-1981), preacher and author: papers (Dr D Martyn Lloyd-Jones Papers)
- Bernice Ruth Rubens (b 1927), novelist: papers (Bernice Rubens Literary Papers)
- Frances Louise Stevenson (1888-1972), personal secretary and second wife of David Lloyd George: corresp and papers (Frances Stevenson Family Papers)
- Brinley Thomas (1906-94), Professor of Economics, Cardiff University: corresp and papers (Professor Brinley Thomas Papers)
- Eirene Lloyd White (1909-99), Baroness White of Rhymney, politician: papers (Eirene White Papers)
- John Ellis Caerwyn Williams (1912-99), scholar, editor, Professor of Irish at University of Wales, Aberystwyth: papers (Papurau J.E. Caerwyn Williams)
- Celtic League: records 1963-91 (Celtic League Records)
- Gweled (Welsh Association of Visual Arts): adminstrative records 1984-98 (Archif Gweled)
- Labour Party Wales (addnl): records (Labour Party Wales Records)
- Liberal Democrats Wales: records 1984-99 (Liberal Democrats Wales Records)
- Made In Wales Stage Company: scripts of productions, commissions and workshops 1981-95 (Made In Wales Stage Company Records)
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National Library of Wales